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References 55 — 65 Abstract Nanostructured carbon materials with large surface area and desired chemical functionalities have been attracting considerable attention because of their extraordinary physicochemical properties and great application potentials in catalysis, environment, and energy storage.
However, the traditional approaches to fabricating these materials rely greatly on complex procedures and specific precursors.
We present a simple, effective, and scalable strategy for the synthesis of functional carbon materials by transition metal—assisted carbonization of conventional small organic molecules. We demonstrate that transition metals can promote the thermal stability of molecular precursors and assist the formation of thermally stable polymeric intermediates during the carbonization process, which guarantees the successful preparation of carbons with high yield.
The versatility of this synthetic strategy allows easy control of the surface chemical functionality, porosity, and morphology of carbons at the molecular level. Furthermore, the prepared carbons exhibit promising performance in heterogeneous catalysis and electrocatalysis.
In particular, when CMs have high surface area, porous structure, and the desired heteroatom doping, their performance in certain applications becomes especially outstanding and competitive 6 — 9.
Traditionally, CMs were prepared by the carbonization of low—vapor pressure natural products, such as cellulose 3 , 13 , chitin 14 , starch 15 , alginic acid 16 , and chitosan 17 , and synthetic polymers, such as polyacrylonitrile 18 , polyaniline 11 , and phenolic resins 6 , The main drawback of natural precursors for CM synthesis is the difficulty to tailor the microstructures and chemical compositions of the obtained products because of the poor solubility and limited heteroatom contents and species in natural precursors.
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